原位氧化FeNiMnAlCrC高熵合金的光热转换性能

材料科学与工程

原位氧化FeNiMnAlCrC高熵合金的光热转换性能

李雨洁，

章飞，

陈梅洁，

李开洋，

熊志平，

宋旼，

王章维

中国有色金属学报

第34卷, 第11期

pp.3595-3607

纸质出版 2024-11-28

DOI：10.11817/j.ysxb.1004.0609.2024-45082

中图分类号：TG139

7900

本文采用经济的原位氧化和选择性刻蚀工艺，通过调控氧化温度和表面粗糙度，研究了Fe₄₀Ni₁₁Mn₃₅Al₇Cr₆C₁(摩尔分数，%)高熵合金表面的氧化产物变化及其对太阳能光热转换性能的影响。结果表明：在500~700 ℃范围内，随着温度升高和刻蚀引起的初始表面粗糙度的增大，氧化后高熵合金表面的氧化物尺寸、氧化层厚度、粗糙度和氧化物种类均呈上升趋势，使得光热转换性能逐渐提升。预先刻蚀并经700 ℃氧化2 h后，合金的太阳能吸收率和光热转换效率分别达到峰值90.4%和87.9%。当氧化温度继续升高至800 ℃后，由于热膨胀系数不匹配导致热应力增大，合金表面生成的氧化层均开始大面积脱落，进而导致材料的光热性能开始下降。本研究为金属氧化层的有效设计提供了理论支持，有助于实现高熵合金光热性能的优化与提升。

高熵合金原位氧化选择性刻蚀光热转换太阳能选择性吸收材料

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